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JAEA Reports

Preparation of waste standards; Annual report 2022

Project Promotion Department; Radioactive Wastes Disposal Center

JAEA-Review 2023-037, 162 Pages, 2024/02

JAEA-Review-2023-037.pdf:2.66MB

For near surface disposal of radioactive wastes generated from research, industrial and medical facilities, Japan Atomic Energy Agency has discussed methods for corresponding to the technical standards on confirmation related to waste disposal, etc. From FY2022, we have established Waste Standards Committee and interim Waste Acceptance Criteria, Waste Package Confirmation Procedure, etc. have been considered. In FY2022, Waste Package Confirmation Procedures of solidified liquid waste and cement filled waste and related standards were discussed. In addition, issues of preparation of Waste Package Confirmation Procedure and rational treatment method for decommissioning wastes were considered. This annual report summarizes the results of discussion in FY2022.

Journal Articles

Circumstances of establishment of regulations for near surface disposal of radioactive waste generated from research facilities, etc.

Sakai, Akihiro

Dekomisshoningu Giho, (64), p.24 - 33, 2023/05

Japan Atomic Energy Agency (JAEA) has proceeded with the project of near surface disposal of radioactive waste generated from research facilities, etc. as the implementing body. On the other hand, Nuclear Regulation Authority (NRA) has established the safety regulations and standards for the operation of the disposal facilities. This report outlines the disposal project of JAEA and the development of the regulations and standards for the disposal by NRA.

Journal Articles

Status of technical development for near surface disposal of radioactive waste generated from research facilities, etc.

Sakai, Akihiro

Dai-33-Kai Genshiryoku Shisetsu Dekomisshoningu Gijutsu Koza Tekisuto, p.31 - 63, 2023/02

The Japan Atomic Energy Agency (JAEA) is promoting the project for concrete-vault disposal and landfill-type disposal of radioactive waste generated from research facilities, etc. This report introduces current status of technical development for JAEA's disposal project as following items; (1) kinds of research facilities and characteristics of radioactivity inventory of the waste, (2) the structures of the disposal facilities which JAEA conceptually designed, (3) development of waste acceptance criteria for major radioactive waste for the JAEA disposal facilities, (4) the concept of the criteria for disposal of uranium bearing waste, that has been established in 2021.

Journal Articles

Disposal project for LLW and VLLW generated from research facilities in Japan; A Feasibility study for the near surface disposal of VLLW that includes uranium

Sakai, Akihiro; Hasegawa, Makoto; Sakamoto, Yoshiaki; Nakatani, Takayoshi

Proceedings of International Conference on the Safety of Radioactive Waste Management (Internet), p.98_1 - 98_4, 2016/11

The radioactivity of uranium-bearing waste contaminated by refined uranium increases with the production of its progeny on a long-term timescale. Therefore, the long-term safety concept of the near surface disposal of uranium-bearing waste is very important. The Japan Atomic Energy Agency (JAEA) examines disposal safety by controlling the average uranium radioactivity concentration in each section of disposal facility and performing safety assessment for very conservative assumptions.

Journal Articles

Characterization of F$$^{+}$$-irradiated graphite surfaces using photon-stimulated desorption spectroscopy

Sekiguchi, Tetsuhiro; Baba, Yuji; Shimoyama, Iwao; Nath, K. G.

Surface and Interface Analysis, 38(4), p.352 - 356, 2006/04

 Times Cited Count:3 Percentile:7.13(Chemistry, Physical)

We investigated the orientation nature at the top-most layers of F$$^{+}$$-irradiated graphite using polarization dependent near-edge X-ray absorption fine structure (NEXAFS) spectroscopy which incorporates partial electron yield (PEY) detection and photon-stimulated ion desorption (PSID) techniques. The fluorine K-edge NEXAFS spectra conducted in PEY mode show no significant dependence on polarization angles. In contrast, NEXAFS spectra recorded in F$$^{+}$$ ion yield mode show enhanced yields at a feature of $$sim$$689.4 eV assigned as a $$sigma$$*(C-F) state relevant to =C-F sites, which depend on polarization angles. The C-F bonds prefer relatively tilting down the surface at the top-most layer, while the C-F bonds are randomly directed at deeper regions. We conclude that the difference in the orientation structures between the top surface and bulk is reflected in the NEXAFS recorded in the two different detection modes. It was also found that H$$^{+}$$- and F$$^{2+}$$- PSID NEXAFS spectra are helpful in understanding desorption mechanism, thus in analysing NEXAFS data.

Journal Articles

Mechanism of state-specific enhancement in photon-stimulated desorption as studied using a polarization-dependent technique

Sekiguchi, Tetsuhiro; Baba, Yuji; Shimoyama, Iwao; Wu, G.*; Kitajima, Yoshinori*

Surface Science, 593(1-3), p.310 - 317, 2005/11

 Times Cited Count:2 Percentile:11.64(Chemistry, Physical)

Using a newly developed rotatable time-of-flight mass spectrometer(R-TOF-MS) and polarized synchrotron radiation, orientation effect on fragmentation and desorption pathways occurring at the top-most layers of molecular solids have been investigated. Reported will be polarization-angle dependencies of TOF mass spectra, high-resolution electron- and ion-NEXAFS in condensed chlorobenzene.

Journal Articles

Direct and indirect processes in photon-stimulated ion desorption from condensed formamide

Ikeura, Hiromi*; Sekiguchi, Tetsuhiro; Baba, Yuji; Imamura, Motoyasu*; Matsubayashi, Nobuyuki*; Shimada, Hiromichi*

Surface Science, 593(1-3), p.303 - 309, 2005/11

 Times Cited Count:5 Percentile:26.1(Chemistry, Physical)

no abstracts in English

Journal Articles

Substitution effect on orientation of organosilicon compounds (CH$$_{3}$$)$$_{3}$$SiX (X = F, Cl, Br, I, NCO) as studied using NEXAFS spectroscopy

Sekiguchi, Tetsuhiro; Baba, Yuji; Shimoyama, Iwao; Nath, K. G.*; Uddin, M. N.*

Journal of Physics; Condensed Matter, 17(36), p.5453 - 5466, 2005/09

 Times Cited Count:1 Percentile:6.21(Physics, Condensed Matter)

The orientation nature of multilayer organosilicon compounds has been investigated by measuring the dependence of the Si K-shell near-edge X-ray absorption fine structures (NEXAFS) on the polarization angle. Two approaches helped to elucidate the orientation mechanism: the substitution effect and the deposition-rate dependence. The orientation angles of Si-X bond axes were obtained for trimethylsilyl halides, (CH$$_{3}$$)$$_{3}$$SiX (X =F Cl Br I NCO, condensed on Cu(111) at a low (82 K) temperature: the angles are 60, 73, 61, 55, and 55 degrees with respect to the surface normal, for X =F, Cl, Br, I, and NCO, respectively. Chloride (X =Cl) produces the most parallel tilt angle. The specific orientation nature of chloride is attributed to its strong dipole moment as well as the regular tetrahedron shape of the molecule. The molecular volumes calculated verify this view. Furthermore, deposition rates are found to greatly influence the growth manner: namely, high deposition rates led to a slightly perpendicular orientation of Si-X bond axis.

Journal Articles

Electronic structure and the Fermi surface of PuCoGa$$_5$$ and NpCoGa$$_{5}$$

Maehira, Takahiro; Hotta, Takashi; Ueda, Kazuo; Hasegawa, Akira*

Physical Review Letters, 90(20), p.207007_1 - 207007_4, 2003/05

 Times Cited Count:94 Percentile:92.38(Physics, Multidisciplinary)

By using a relativistic linear augmented-plane-wave method, we clarify energy band structures and Fermi surfaces of recently discovered plutonium-based superconductor PuCoGa$$_5$$. We find several cylindrical sheets of Fermi surfaces with large volume, quite similar to CeMIn$$_5$$ (M=Ir and Co) isostructural with PuCoGa$$_5$$, in spite of different $$f$$-electron numbers between Ce$$^{3+}$$ and Pu$$^{3+}$$ ions. This similarity is simply understood by a concept of electron-hole conversion in a tight binding model constructed based on the $$j$$-$$j$$ coupling scheme. Due to the present results, we provide a possible scenario to explain why a transition temperature is so high as 18.5K in PuCoGa$$_5$$.

Journal Articles

Relativistic band-structure calculations for CeTIn$$_5$$(T=Ir and Co) and analysis of the energy bands by using tight-binding method

Maehira, Takahiro; Hotta, Takashi; Ueda, Kazuo; Hasegawa, Akira*

Journal of the Physical Society of Japan, 72(4), p.854 - 864, 2003/04

 Times Cited Count:75 Percentile:90.21(Physics, Multidisciplinary)

In order to investigate electronic properties of recently discovered heavy fermion superconductors CeTIn$$_5$$ (T=Ir and Co), we employ the relativistic linear augmented-plane-wave (RLAPW) method to clarify the energy band structures and Fermi surfaces of those materials.The obtained energy bands mainly due to the large hybridization between Ce $$4f$$ and In 5$$p$$ states well reproduce the Fermi surfaces consistent with the de Haas-van Alphen experimental results. For the purpose, we construct a tight-binding model for CeTIn$$_5$$ by including $$f$$-$$f$$ and $$p$$-$$p$$ hoppings as well as $$f$$-$$p$$ hybridization, which are expressed by the Slater-Koster integrals, determined by the direct comparison with the band-calculation result. Similarity and difference between CeIrIn$$_5$$ and CeCoIn$$_5$$ are discussed based on the obtained tight-binding model, suggesting a significant importance of the effect of crystalline electric field to understand the difference in electronic properties among CeTIn$$_5$$.

Journal Articles

Free surface shear layer instabilities on a high-speed liquid jet

Ito, Kazuhiro*; Tsuji, Yoshiyuki*; Nakamura, Hideo; Kukita, Yutaka*

Fusion Technology, 37(1), p.74 - 88, 2000/01

no abstracts in English

Journal Articles

Initial free surface instabilities on a high speed water jet simulating a liquid-metal target

Ito, Kazuhiro*; Tsuji, Yoshiyuki*; Nakamura, Hideo; Kukita, Yutaka*

Fusion Technology, 36(1), p.69 - 84, 1999/07

no abstracts in English

Journal Articles

Near surface disposal of very low level waste generated from reactor decommissioning and related safety requirements

Okoshi, Minoru; Yoshimori, Michiro; Abe, Masayoshi

Planning and Operation of Low Level Waste Disposal Facilities IAEA-SM-341/70, 0(0), p.416 - 425, 1997/00

no abstracts in English

Journal Articles

Safety demonstration test for the disposal of very low level concrete waste

Abe, Masayoshi; Okoshi, Minoru; Yoshimori, Michiro

Dekomisshoningu Giho, 0(15), p.50 - 58, 1996/12

no abstracts in English

Journal Articles

Near surface disposal of VLLW from reactor decommissioning and safety requirements

Okoshi, Minoru; Yoshimori, Michiro

Proc. of 3rd Japan-Russia Joint Symp. on Radiation Safety, 0, p.75 - 85, 1995/00

no abstracts in English

JAEA Reports

Reflood experiments in single rod channel under high-pressure condition

G.Xu*; Kumamaru, Hiroshige; Tasaka, Kanji

JAERI-M 89-178, 35 Pages, 1989/11

JAERI-M-89-178.pdf:0.74MB

no abstracts in English

Oral presentation

Outline of the disposal of very low level concrete waste in JAEA

Tsuji, Tomoyuki

no journal, , 

Japan Atomic Energy Agency (JAEA), who conducted the demonstration test on a safe dismantling of Japan Power Demonstration Reactor (JPDR) in Nuclear Science Research Institute, has been performing the safe demonstration test of near-surface disposal of very low level (VLL) concrete waste arising from JPDR dismantling. Approximately 1,700 tons of VLL concrete wastes were placed in a simple disposal facility, of which dimensions are 45 m$$times$$16 m and 3.5 m in depth without any engineered barrier, and covered with soil of 2.5 m thickness. The safe demonstration test of near-surface disposal of VLL concrete waste consists of a operation stage (FY 1995-1996) and a management stage (FY 1996-2024). In the operation stage, radiation dose around the disposal facility was measured, and radioactivity concentrations in groundwater and soil were analyzed. After we proceeded the management stage of disposal, radiation monitoring was continued additionally for 3 years in the management stage. An inspection such as no outflow, crack and subsidence of the covered soil is conducted at once a week. The radiation monitoring data is planned to storage properly by management department until the finishing of management stage, and an inspection data is stored in accordance with the Act on the Regulation of Nuclear Source Material, Nuclear Fuel Material and Reactors.

Oral presentation

Disposal project of low-level radioactive waste generated from research facilities, etc.; Development for impermeable function of cover soil of trench disposal facility

Sakai, Akihiro

no journal, , 

Japan Atomic Energy Agency (JAEA) is promoting the project for near surface disposal of low-level radioactive waste generated from research facilities, etc. Since a function to reduce infiltration water into the cover soil is needed at trench facilities for very low-level waste, we are calculating the infiltration water through the cover soil which is installed in various composition and parameters of the impermeable sheet, low permeable soil layer and drainage layer by using the HELP code developed by EPA and a calculation code by two-dimensional finite element method. This report outlines these studies that have been conducted on the impermeable function of the trenching facilities.

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